My list:
1. Grant Ward
2. Loki
3. Kingpin
4. Alexander Pierce
5. Ultron
6. Obadiah Stane
7. Red Skull
8. Abomination
9. Yellow Jacket
10. Ronan
I don't consider Winter Soldier a villain, more like a force since he was being controlled. Most of these villains have been subpar, except for the top 3/4. I hope we get some great villains in the future, such as Purple Man and Baron Zemo.
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