Harley really does have a mean streak, but she certainly wavers in her sense of evil. She would probably fit in well with the secret six, in that she has some sort of moral code, albeit flexible, and will show heavy remorse for some of her actions. But if things get out of hand, or if she has to, she has no problem getting fatal.
Ivy just has her own agenda and does not care about how much she hurts of manipulates others, and if she lingers on it, it isn't for long. I think this is only worsened by her latest outing with Clayface, which is the first time ever that I found Clayface compelling because of how betrayed he was at Ivy's hands. I blame it on her roots to the plant world, which dehumanizes her a bit. But in the end, Ivy is definitely more cruel.
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