In your opinion, who are the most developed and complex villains in the entire Marvel Cinematic Universe?
Kingpin, Kilgrave, and Grant Ward have had the benefit of TV episodes to flesh them out, so I'd say they take the cake for most complex and developed
Loki also is up there, due to being in several movies, but he still does the same thing every appearance. "Ah, I'm evil! Wait, jk I'm good! Wait, jk jk I'm actually evil! Wait, jk jk jk I'm good, and will seemingly sacrifice myself for the greater good! Jk x4, I'm alive!"
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