He'd not that smart through. The bloody comic relief was able to be a better detective than him. Hell, if we take the leaks into account he's just Eobard putting on a stupid accent and hiding in plain sight.
The only way Zemo found out was through prior connections and a burning desire to ruin the Avengers- a week with money isn't going to cut it.
No. Sherloque is a buffoon with very little actual detective feats. There's no reason to assume he could figure out an actually well hidden secret like Bucky's assassination records.
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