Of the characters I do know (Light, L, Conan, Batman and Lex Luthor), it just depends. These characters are ruthless in their intelligence. Meruem adapts every time he loses, finding out the subconscious pattern in whatever they're doing. So Meruem would eventually beat all of them. The issue is, he'd have to lose a couple times before figuring it out, and these enemies are pretty careful not to overlook such a flaw.
Komugi has a nen ability and condition to never lose at Gungi. I truly believe that after years and years of playing, Meruem would eventually beat Gungi. None of these characters have that advantage.
@back_stabbath95: Not sure he would be able to do much of anything against her considering he uses illegal cards and makes up most of the rules to the game XD
@bobandjim1260: yugi/kaiba screws the rules is fantastic. Though in the manga the whole first volume has nothing to do with duel monsters and is rather yami going around challenging criminals to random games and he f***s with people lol
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