Neal Adams appears in 32 issues in this volume.
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Issue #143
The Big Fall ; Superboy's Civil War Time Trip!
December 1, 1967
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Issue #145
The Fantastic Faces! ; Superboy Meets William Tell!
March 1968
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Issue #146
The Runaway Superboy! ; The Superboy Legend ; The Notorious Captain Sinbad Kent!
April 1, 1968
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Issue #147
The Origin of the Legion
June 1, 1968
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Issue #148
Superboy's Greatest Gamble! ; The Canine that Outclassed Krypto!
June 1968
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Issue #149
Wanted: Dead or Alive Bonnie Lang and Clyde Kent! ; The Great Super-Powers Contest!
July 1968
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Issue #150
The Stranger Who Stalks Smallville!
September 1, 1968
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Issue #151
D.O.A. - In Cold Blood
October 1, 1968
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Issue #152
The 2 Faces of Superboy!
December 1, 1968
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Issue #153
Challenge of the Cosmic Invaders ; Superboy's Secret Hideaways
January 1, 1969
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Issue #154
Blackout for Superboy!
March 1, 1969
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Issue #155
Revolt of the Teen-Age Robots!
April 1, 1969
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Issue #157
Get Lost, Superboy ... Who Needs You? ; How the Super-Family Came to Earth from Krypton ; Special 100th Anniversary Souvenirs
June 1, 1969
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Issue #158
Superboy's Darkest Secret!
July 1, 1969
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Issue #159
The Day It Rained Superboys!
September 1969
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Issue #160
I Chose External Exile!
October 1, 1969
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Issue #161
The Strange Death of Superboy! ; More of Superboy's Secret Hideaways
December 1, 1969
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Issue #163
Reform School Rebel
March 1, 1970
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Issue #164
Your Death Will Destroy Me!
April 1, 1970
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Issue #166
Here Lies the Real Superboy! ; The Kryptonite Conqueror!
June 1, 1970
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Issue #167
The Day Superbaby Blew Up the World! ; The Super-Mammoth Mystery!
July 1, 1970
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Issue #168
Leave Us ... Or We Perish! ; The Negative Boy of Steel
September 1, 1970
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Issue #170
Easy Rider to Doom ; Superboy's Biggest Blunder!
December 1, 1970
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Issue #172
The World of the Super-Ape! / Brotherly Hate!
March 1, 1971
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Issue #173
The Super-Clark of Smallville! ; Trust Me or Kill Me!
April 1, 1971
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Issue #175
Doomsday for a Super-Phantom!
June 1, 1971
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Issue #176
The Secret of Superboy's Sister ; Invisible Invader!
July 1, 1971
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Issue #177
Our Traitor Super-Son ; Plague from the Past ; The Revenge of the Knave from Krypton!
September 1, 1971
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Issue #178
Pawn of the Monster Maker ; The Lone Wolf Legionnaire ; Kryptonite ; Superbaby's First Friend!
October 1, 1971
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Issue #205
The Legion of Super-Executioners
December 1, 1974
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Issue #215
The Final Eclipse Of Sun Boy
March 1, 1976
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Issue #216
The Hero Who Hated The Legion ; 1 [plus] 1 = 3
April 1, 1976
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